Lynn Kamerlin
Professor
Evolution of chalcone isomerase from a noncatalytic ancestor
Author
Summary, in English
The emergence of catalysis in a noncatalytic protein scaffold is a rare, unexplored event. Chalcone isomerase (CHI), a key enzyme in plant flavonoid biosynthesis, is presumed to have evolved from a nonenzymatic ancestor related to the widely distributed fatty-acid binding proteins (FAPs) and a plant protein family with no isomerase activity (CHILs). Ancestral inference supported the evolution of CHI from a protein lacking isomerase activity. Further, we identified four alternative founder mutations, i.e., mutations that individually instated activity, including a mutation that is not phylogenetically traceable. Despite strong epistasis in other cases of protein evolution, CHI's laboratory reconstructed mutational trajectory shows weak epistasis. Thus, enantioselective CHI activity could readily emerge despite a catalytically inactive starting point. Accordingly, X-ray crystallography, NMR, and molecular dynamics simulations reveal reshaping of the active site toward a productive substrate-binding mode and repositioning of the catalytic arginine that was inherited from the ancestral fatty-acid binding proteins.
Publishing year
2018-06
Language
English
Pages
548-555
Publication/Series
Nature Chemical Biology
Volume
14
Issue
6
Document type
Journal article
Publisher
Nature Publishing Group
Keywords
- Catalysis
- Catalytic Domain
- Chalcones/genetics
- Cloning, Molecular
- Crystallography, X-Ray
- Epistasis, Genetic
- Escherichia coli
- Evolution, Molecular
- Fatty Acid-Binding Proteins/chemistry
- Flavonoids/chemistry
- Genes, Plant
- Intramolecular Lyases/genetics
- Kinetics
- Magnetic Resonance Spectroscopy
- Models, Molecular
- Molecular Dynamics Simulation
- Mutation
- Phylogeny
- Plant Proteins/metabolism
- Plants/metabolism
- Protein Conformation
Status
Published
ISBN/ISSN/Other
- ISSN: 1552-4469